One-minute synthesis of crystalline microporous aluminophosphate (AlPO4-5) by combining fast heating with a seed-assisted method.

نویسندگان

  • Zhendong Liu
  • Toru Wakihara
  • Daisuke Nishioka
  • Kazunori Oshima
  • Takahiko Takewaki
  • Tatsuya Okubo
چکیده

Herein, we report a rapid route for the synthesis of AlPO4-5. By combining fast heating in a tubular reactor with a seed-assisted method, both of which were found to be crucial, the preparation of AlPO4-5 was completed in one minute, making this route the fastest known for the preparation of the crystalline microporous materials.

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Nano-sized AlPO4-5 Crystals: Synthesis and characterization

Molecular sieves and zeolites are materials whose crystalline frameworks form nanometer or subnanometer pores. A variety of different crystal structures are known having a range of pore sizes. Because the pore sizes are usually smaller than 2 nm, they are classified as microporous materials. Synthesis of microporous materials is usually conducted by the high temperature treatment (80-200 °C) of...

متن کامل

Nano-sized AlPO4-5 Crystals: Synthesis and characterization

Molecular sieves and zeolites are materials whose crystalline frameworks form nanometer or subnanometer pores. A variety of different crystal structures are known having a range of pore sizes. Because the pore sizes are usually smaller than 2 nm, they are classified as microporous materials. Synthesis of microporous materials is usually conducted by the high temperature treatment (80-200 °C) of...

متن کامل

The selective adsorption of tellurium in the aluminosilicate regions of AFI- and MOR-type microporous crystals.

Attempts have been made to load tellurium (Te) atoms into the one-dimensional nano-channels of microporous crystals of aluminophosphate AlPO4-5 and of aluminosilicate mordenites of the Na(+) form (Na-MOR) and the H(+)-form (H-MOR) at 673 K. The density of the atoms adsorbed was in the sequence 0 ∼ AlPO4-5 ≪ H-MOR < Na-MOR. AlPO4-5 provides a shallow potential of periodical charge fluctuation fo...

متن کامل

Simulation of Alkane Adsorption in the Aluminophosphate Molecular Sieve AlPO4-5

Adsorption isotherms of alkanes ranging from methane through pentane in the microporous aluminophosphate AlPO4-5 are calculated using grand canonical monte carlo simulations. These simulations predict a surprisingly complex behavior. For methane and ethane we find at low temperatures a low-density-high-density transition that resembles capillary condensation. At intermediate temperatures a high...

متن کامل

Microwave Assisted Synthesis of Nano Zeolite Seed for Synthesis Membrane and Investigation of its Permeation Properties for H2 Separation

MFI-type zeolite membranes (ZSM-5) were prepared on α-alumina tubular supports and tested for separation of H2/CO mixtures. The effect of pressure and temperature on H2 and CO flows and selectivity was investigated. The best results in this work were obtained with a ZSM-5 membrane prepared over a porous α-alumina tube seeded with zeolite nanocrystals synthesized with m...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

عنوان ژورنال:
  • Chemical communications

دوره 50 19  شماره 

صفحات  -

تاریخ انتشار 2014